Source code for amorphgen.pipeline.quench

"""
amorphgen.pipeline.quench
--------------------------
Stage 5 – Cool the melt from T_start down to T_end via a temperature ramp.

Ensemble is configurable: NVT (default) or NPT.
"""

from __future__ import annotations

from copy import deepcopy
from ase.io import read, write
from ase.md.velocitydistribution import MaxwellBoltzmannDistribution

from ..utils import (get_calculator, build_md_dynamics,
                     attach_outputs, merge_config)
from ..configs import DEFAULT_CONFIG


[docs] def run(atoms_or_file, cfg_override=None, calc=None, **kwargs): """ Cool the structure from T_start -> T_end. Parameters ---------- atoms_or_file : str or ase.Atoms cfg_override : dict, optional calc : ASE calculator, optional Returns ------- ase.Atoms — quenched structure at T_end """ global_cfg = merge_config(DEFAULT_CONFIG, cfg_override) cfg = global_cfg["quench"] ensemble = cfg.get("ensemble", "NVT").upper() if isinstance(atoms_or_file, str): atoms = read(atoms_or_file) print(f"[Stage 5] Loaded from {atoms_or_file}") else: atoms = deepcopy(atoms_or_file) print("[Stage 5] Using provided Atoms object") logfile = cfg.get("log_file", "stage5_quench.log") trajfile = cfg.get("traj_file", "stage5_quench_traj.xyz") # Frame-level resume: continue a walltime-killed quench from the last # trajectory frame (momenta included); ramp position recovered via # ramp_resume_position. The legacy filename lets a run interrupted # under a pre-rename AmorphGen still resume after upgrade. from ..utils.common import (resume_md_stage, needs_velocity_init, ramp_resume_position) ck_atoms, elapsed = resume_md_stage(trajfile, kwargs.get("resume"), "5", legacy_trajfile="stage5_quench.xyz") if ck_atoms is not None: atoms = ck_atoms if calc is None: from ..utils.common import resolve_device device = resolve_device(global_cfg.get("device", "cuda")) calc = get_calculator( model=global_cfg.get("model", "mace-mpa-0"), device=device, model_path=global_cfg.get("model_path"), ) atoms.calc = calc T_start = cfg["T_start"] if needs_velocity_init(atoms, elapsed): MaxwellBoltzmannDistribution(atoms, temperature_K=T_start) dyn = build_md_dynamics( atoms, ensemble=ensemble, T=T_start, timestep=cfg.get("timestep", 1.0), friction=cfg.get("friction", 0.01), ttime=cfg.get("ttime", 25.0), npt_method=cfg.get("npt_method", "berendsen"), taup_factor=cfg.get("taup_factor", 10.0), compressibility_GPa=cfg.get("compressibility_GPa", 100.0), ) logger, traj = attach_outputs(dyn, atoms, logfile, trajfile, fmt=global_cfg.get("traj_format", "extxyz"), append=elapsed > 0) T_end = cfg["T_end"] T_step = cfg.get("T_step", -100) timestep_fs = cfg.get("timestep", 1.0) # Allow rate (K/ps) to auto-calculate steps_per_T rate = cfg.get("rate") if rate is not None: steps = int(round(abs(T_step) / (rate * timestep_fs / 1000))) steps = max(steps, 1) else: steps = cfg.get("steps_per_T", 1000) # Build temperature list (cooling) temps = [] T = T_start while T >= T_end - 1e-6: temps.append(int(round(T))) T += T_step from ..utils.common import compute_density_gcm3 density = compute_density_gcm3(atoms) actual_rate = abs(T_step) / (steps * timestep_fs / 1000) print(f"[Stage 5] {ensemble} quench: {T_start} -> {T_end} K " f"({T_step} K/step, {steps} steps each, {actual_rate:.1f} K/ps) " f"density={density:.2f} g/cm3") # Recover the ramp position on resume: k0 full segments done, offset # steps into segment k0 (see ramp_resume_position for the # elapsed==total edge semantics). k0, offset = ramp_resume_position(elapsed, steps, len(temps)) for idx, T in enumerate(temps): if idx < k0: continue dyn.set_temperature(temperature_K=T) run_steps = steps - offset if idx == k0 else steps note = f" (resumed, {run_steps} steps left)" if (idx == k0 and offset) else "" print(f" -> T = {T:5d} K{note}") dyn.run(run_steps) logger.close() traj.close() out_xyz = cfg.get("output_xyz", "stage5_quenched.xyz") write(out_xyz, atoms, format="extxyz") print(f"[Stage 5] Saved -> {out_xyz}\n") return atoms